#METABOLOMICS WORKBENCH juliehaines_20241125_124620 DATATRACK_ID:5395 STUDY_ID:ST003603 ANALYSIS_ID:AN005919 PROJECT_ID:PR002231
VERSION             	1
CREATED_ON             	December 5, 2024, 7:15 pm
#PROJECT
PR:PROJECT_TITLE                 	Macrophages recycle phagocytosed bacteria to fuel immunometabolic responses
PR:PROJECT_SUMMARY               	Macrophages specialize in phagocytosis, a cellular process that eliminates
PR:PROJECT_SUMMARY               	extracellular matter, including microbes, through internalization and
PR:PROJECT_SUMMARY               	degradation. Despite the critical role of phagocytosis during bacterial
PR:PROJECT_SUMMARY               	infection, the fate of phagocytosed microbial cargo and its impact on host cell
PR:PROJECT_SUMMARY               	is poorly understood. Here, we reveal that ingested bacteria constitute an
PR:PROJECT_SUMMARY               	alternative nutrient source that skews immunometabolic host responses. Tracing
PR:PROJECT_SUMMARY               	stable isotope-labelled bacteria, we found that phagolysosomal degradation of
PR:PROJECT_SUMMARY               	bacteria provides carbon atoms and amino acids that are recycled into various
PR:PROJECT_SUMMARY               	metabolic pathways, including glutathione and itaconate biosynthesis, and
PR:PROJECT_SUMMARY               	satisfy macrophage bioenergetic needs. Metabolic recycling of
PR:PROJECT_SUMMARY               	microbially-derived nutrients is regulated by the nutrient sensing mTORC1 and
PR:PROJECT_SUMMARY               	intricately tied to microbial viability. Dead bacteria, as opposed to live ones,
PR:PROJECT_SUMMARY               	are enriched in cyclic- adenosine monophosphate (AMP), sustain the cellular AMP
PR:PROJECT_SUMMARY               	pool and subsequently activate AMP protein kinase (AMPK) to inhibit mTORC1.
PR:PROJECT_SUMMARY               	Consequently, killed bacteria strongly fuel metabolic recycling and support
PR:PROJECT_SUMMARY               	macrophage survival, but elicit decreased reactive oxygen species (ROS)
PR:PROJECT_SUMMARY               	production and a reduced IL-1β secretion compared to viable bacteria. These
PR:PROJECT_SUMMARY               	results reveal a novel insight into the fate of engulfed microbes and highlights
PR:PROJECT_SUMMARY               	a microbial viability-associated metabolite that triggers host metabolic and
PR:PROJECT_SUMMARY               	immune responses. Our findings hold promise for shaping immunometabolic
PR:PROJECT_SUMMARY               	intervention in various immune-related pathologies.
PR:INSTITUTE                     	University of Colorado Anschutz Medical Campus
PR:LABORATORY                    	Lab of Angelo D'Alessandro in collaboration with lab of Johan Garaude (INSERM,
PR:LABORATORY                    	Fr)
PR:LAST_NAME                     	Haines
PR:FIRST_NAME                    	Julie
PR:ADDRESS                       	12801 E 17th Ave, Room 1303, Aurora, Colorado, 80045, USA
PR:EMAIL                         	julie.haines@cuanschutz.edu
PR:PHONE                         	3037243339
#STUDY
ST:STUDY_TITLE                   	Comparison of metabolic responses in murine bone marrow derived macrophages upon
ST:STUDY_TITLE                   	LPS treatment versus following the engulfment of live or dead E coli.
ST:STUDY_SUMMARY                 	Global metabolomics and 13C-tracing analysis of murine bone marrow derived
ST:STUDY_SUMMARY                 	macrophages exposed to live or heat-killed uniformly 13C-labelled E. coli in a
ST:STUDY_SUMMARY                 	trans-well system for 6h or 18h. Global metabolomics was performed in parallel
ST:STUDY_SUMMARY                 	on murine BMDMs treated with 500 ng/ml LPS for 18h.
ST:INSTITUTE                     	University of Colorado Anschutz Medical Campus
ST:LAST_NAME                     	Haines
ST:FIRST_NAME                    	Julie
ST:ADDRESS                       	12801 E 17th Ave, Room 1303, Aurora, Colorado, 80045, USA
ST:EMAIL                         	julie.haines@cuanschutz.edu
ST:PHONE                         	3037243339
#SUBJECT
SU:SUBJECT_TYPE                  	Cultured cells
SU:SUBJECT_SPECIES               	Mus musculus
SU:GENDER                        	Not applicable
#SUBJECT_SAMPLE_FACTORS:         	SUBJECT(optional)[tab]SAMPLE[tab]FACTORS(NAME:VALUE pairs separated by |)[tab]Raw file names and additional sample data
SUBJECT_SAMPLE_FACTORS           	-	156	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-01
SUBJECT_SAMPLE_FACTORS           	-	157	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-02
SUBJECT_SAMPLE_FACTORS           	-	158	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-03
SUBJECT_SAMPLE_FACTORS           	-	159	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:live | Multiplicity of infection:25	RAW_FILE_NAME(Raw file name)=F2-23-04
SUBJECT_SAMPLE_FACTORS           	-	160	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:live | Multiplicity of infection:25	RAW_FILE_NAME(Raw file name)=F2-23-05
SUBJECT_SAMPLE_FACTORS           	-	161	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:live | Multiplicity of infection:25	RAW_FILE_NAME(Raw file name)=F2-23-06
SUBJECT_SAMPLE_FACTORS           	-	162	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:25	RAW_FILE_NAME(Raw file name)=F2-23-07
SUBJECT_SAMPLE_FACTORS           	-	163	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:25	RAW_FILE_NAME(Raw file name)=F2-23-08
SUBJECT_SAMPLE_FACTORS           	-	164	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:25	RAW_FILE_NAME(Raw file name)=F2-23-09
SUBJECT_SAMPLE_FACTORS           	-	165	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):500 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-10
SUBJECT_SAMPLE_FACTORS           	-	166	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):500 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-11
SUBJECT_SAMPLE_FACTORS           	-	167	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):500 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-12
SUBJECT_SAMPLE_FACTORS           	-	174	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-19
SUBJECT_SAMPLE_FACTORS           	-	175	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-20
SUBJECT_SAMPLE_FACTORS           	-	176	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-21
SUBJECT_SAMPLE_FACTORS           	-	177	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-22
SUBJECT_SAMPLE_FACTORS           	-	178	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-23
SUBJECT_SAMPLE_FACTORS           	-	179	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-24
SUBJECT_SAMPLE_FACTORS           	-	180	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	RAW_FILE_NAME(Raw file name)=F2-23-25
SUBJECT_SAMPLE_FACTORS           	-	181	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	RAW_FILE_NAME(Raw file name)=F2-23-26
SUBJECT_SAMPLE_FACTORS           	-	182	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	RAW_FILE_NAME(Raw file name)=F2-23-27
SUBJECT_SAMPLE_FACTORS           	-	183	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-28
SUBJECT_SAMPLE_FACTORS           	-	184	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-29
SUBJECT_SAMPLE_FACTORS           	-	185	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	RAW_FILE_NAME(Raw file name)=F2-23-30
SUBJECT_SAMPLE_FACTORS           	-	186	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	RAW_FILE_NAME(Raw file name)=F2-23-31
SUBJECT_SAMPLE_FACTORS           	-	187	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	RAW_FILE_NAME(Raw file name)=F2-23-32
SUBJECT_SAMPLE_FACTORS           	-	188	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	RAW_FILE_NAME(Raw file name)=F2-23-33
#COLLECTION
CO:COLLECTION_SUMMARY            	BMDMs were seeded at 2.5E6 cell/well in a non-tissue treated 6-well plate (2
CO:COLLECTION_SUMMARY            	wells per condition) the day before the experiment. To harvest, BMDMs were
CO:COLLECTION_SUMMARY            	washed with cold PBS and harvested with 5 mM EDTA in PBS, frozen as dry cell
CO:COLLECTION_SUMMARY            	pellet, and stored at -80˚C until processing.
CO:SAMPLE_TYPE                   	Macrophages
#TREATMENT
TR:TREATMENT_SUMMARY             	Preparation of macrophages: Murine bone marrow-derived macrophages (BMDMs) were
TR:TREATMENT_SUMMARY             	generated as described previously, in RPMI 1640 supplemented with M-CSF (30%
TR:TREATMENT_SUMMARY             	mycoplasma-free L929 cell supernatant, NCBI Biosample accession # SAMN00155972)
TR:TREATMENT_SUMMARY             	and 10% FBS, plus 100 µg/ml penicillin, 100 µg/ml streptomycin, 10 mM HEPES, 1
TR:TREATMENT_SUMMARY             	nM sodium pyruvate and 50 µM 2-mercaptoethanol (all from Gibco). BMDMs were
TR:TREATMENT_SUMMARY             	used on day 5 to 7 after seeding. Period of differentiation of the cells,
TR:TREATMENT_SUMMARY             	concentration of cells when replating and time-lapse between replating and
TR:TREATMENT_SUMMARY             	stimulation with bacteria were important parameters to maintain metabolic
TR:TREATMENT_SUMMARY             	backgrounds homogenous between experiments. Preparation of viable and killed
TR:TREATMENT_SUMMARY             	U-[13C]Bacteria: ThyA- E. coli were grown overnight with shaking in LB
TR:TREATMENT_SUMMARY             	supplemented with thymidine (500 µg/ml) and trimethoprim (50 µg/ml), diluted
TR:TREATMENT_SUMMARY             	1/40, and grown until log-phase [optical density at 600 nm (OD600) of 0.8-1.2].
TR:TREATMENT_SUMMARY             	Bacteria were washed with phosphate buffer saline (PBS) to remove LB salts
TR:TREATMENT_SUMMARY             	before addition to cells. For labeling of bacteria, 10 µl of an overnight
TR:TREATMENT_SUMMARY             	cultured of thyA- E. coli was added to 20 ml of a filtered M9 minimal medium
TR:TREATMENT_SUMMARY             	salts (Life Technologies) supplemented with 1 mM thiamine, 1 mM MgSO4, 0.1 M
TR:TREATMENT_SUMMARY             	CaCl2, 500 µg/ml thymidine, 50 µg/ml trimethoprim, and 0.5% U-[13C6] glucose
TR:TREATMENT_SUMMARY             	(Campro Scientific). Bacteria were grown for 72h, washed with PBS and subjected
TR:TREATMENT_SUMMARY             	to heat-killing by re-suspension in PBS and subsequently incubation at 60˚C for
TR:TREATMENT_SUMMARY             	60-90 min. For antibiotic killing, bacteria were incubated for 6h to 12h with
TR:TREATMENT_SUMMARY             	Streptomycin or Gentamycin (50 µg/ml). Bacteria were kept at 4˚C until use.
TR:TREATMENT_SUMMARY             	Efficient killing was confirmed by overnight plating on LB-agar plates.
TR:TREATMENT_SUMMARY             	Treatment of macrophages: 2E6 BMDMs were plated 12-16h prior to stimulation in
TR:TREATMENT_SUMMARY             	6-well plate and insert of a trans-well system (Falcon). Cells in wells were
TR:TREATMENT_SUMMARY             	stimulated with live or killed labelled-E. coli at MOI 50 or with 500 ng/mL LPS.
TR:TREATMENT_SUMMARY             	Cells in inserts were left untreated. Plates were centrifuged at 2000 rpm for
TR:TREATMENT_SUMMARY             	5min. BMDMs were incubated for 5 min and washed with PBS to remove non-ingested
TR:TREATMENT_SUMMARY             	bacteria and further incubated for 6h or 18h.
#SAMPLEPREP
SP:SAMPLEPREP_SUMMARY            	Metabolites from frozen pellets were extracted at 4e6 cells per mL using ice
SP:SAMPLEPREP_SUMMARY            	cold 5:3:2 methanol:acetonitrile:water (v/v/v) with vigorous vortexing at 4
SP:SAMPLEPREP_SUMMARY            	degrees C followed by centrifugation as described for 10 min at 18,000 g.
SP:SAMPLEPREP_SUMMARY            	Supernatants were maintained at 4°C until analysis that same day.
SP:PROCESSING_STORAGE_CONDITIONS 	4℃
SP:EXTRACT_STORAGE               	-80℃
#CHROMATOGRAPHY
CH:CHROMATOGRAPHY_SUMMARY        	Negative C18
CH:CHROMATOGRAPHY_TYPE           	Reversed phase
CH:INSTRUMENT_NAME               	Thermo Vanquish
CH:COLUMN_NAME                   	Phenomenex Kinetex C18 (150 x 2.1mm,1.7um)
CH:SOLVENT_A                     	95% water/5% acetonitrile; 1 mM ammonium acetate
CH:SOLVENT_B                     	95% acetonitrile/5% water; 1 mM ammonium acetate
CH:FLOW_GRADIENT                 	0-0.5 min 0% B, 0.5-1.1 min 0-100% B, 1.1-2.75 min hold at 100% B, 2.75-3 min
CH:FLOW_GRADIENT                 	100-0% B, 3-5 min hold at 0% B
CH:FLOW_RATE                     	450 uL/min
CH:COLUMN_TEMPERATURE            	45
CH:SAMPLE_INJECTION              	6 uL
#ANALYSIS
AN:ANALYSIS_TYPE                 	MS
#MS
MS:INSTRUMENT_NAME               	Thermo Q Exactive Orbitrap
MS:INSTRUMENT_TYPE               	Orbitrap
MS:MS_TYPE                       	ESI
MS:ION_MODE                      	NEGATIVE
MS:MS_COMMENTS                   	Resolution 70,000, scan range 65-900 m/z, maximum injection time 200 ms,
MS:MS_COMMENTS                   	microscans 2, automatic gain control (AGC) 3 x 10^6 ions, source voltage 4.0 kV,
MS:MS_COMMENTS                   	capillary temperature 320 C, and sheath gas 45, auxiliary gas 15, and sweep gas
MS:MS_COMMENTS                   	0 (all nitrogen). Data converted to mzXML using RawConverter. Metabolites were
MS:MS_COMMENTS                   	annotated and integrated using Maven in conjunction with the KEGG database.
#MS_METABOLITE_DATA
MS_METABOLITE_DATA:UNITS	peak area
MS_METABOLITE_DATA_START
Samples	156	157	158	159	160	161	162	163	164	165	166	167	174	175	176	177	178	179	180	181	182	183	184	185	186	187	188
Factors	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:live | Multiplicity of infection:25	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:live | Multiplicity of infection:25	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:live | Multiplicity of infection:25	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:25	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:25	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:25	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):500 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):500 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):500 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):6 | LPS treatment (ng/ml):0 | E coli viability:NA | Multiplicity of infection:NA	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50	Sample source:murine macrophage cells | Timepoint (h):18 | LPS treatment (ng/ml):0 | E coli viability:dead | Multiplicity of infection:50
ADP	3325.88	6094.56	5070.51	23642.66	13655.08	17981.41	25408.77	21666.65	8456.18	13665.28	37090.48	6564.41	77963.41	20680.91	48109.64	8494.28	59597.50	32929.81	13532.66	12864.10	65688.12	7418.63	4129.94	39348.91	23324.42	102714.10	40206.14
AMP	1001673.00	1100723.00	822872.00	1367524.00	1369014.00	1540425.00	1634320.00	1417202.00	1600770.00	1556888.00	1696113.00	1459889.00	3491144.00	3167641.00	3821510.00	757712.20	712339.70	1102771.00	2750876.00	2859514.00	2621580.00	1020398.00	655062.40	1533509.00	2111118.00	1833200.00	1929990.00
GMP	497359.10	559415.40	390626.50	694604.10	563652.70	632060.80	752916.20	964089.30	813336.30	695471.20	735903.50	621930.80	652886.20	765374.50	735555.50	75747.73	143672.00	128792.00	880378.50	1049524.00	957525.50	104735.10	86017.27	127544.20	439809.60	392321.40	356686.00
UMP	677375.10	698854.10	661183.70	688831.40	658433.30	712705.00	757924.80	886917.10	957348.20	557418.20	536974.30	843102.80	916846.30	894049.80	1094206.00	122973.80	233836.80	185984.40	1913829.00	2248918.00	1824518.00	278306.40	180719.80	301831.20	591984.20	489115.20	671505.40
IDP	242201.50	186609.70	178291.90	271857.80	183030.30	385760.60	283016.40	301682.60	574438.30	315456.50	316360.70	456783.50	480336.20	424438.90	353736.90	239142.40	481292.70	309359.50	423544.60	511840.80	313224.50	224020.40	323958.30	521022.50	348183.70	294384.50	831783.80
IMP	718317.70	840200.60	476623.50	1023190.00	730242.20	713092.60	791450.30	1039466.00	714079.90	532254.70	676041.90	640946.80	829746.40	1245912.00	860056.80	75527.80	117495.00	136240.10	490469.20	600303.00	497147.20	80136.95	92716.74	115946.30	380186.50	414395.20	453201.90
Inosine	1781989.00	2457493.00	1918905.00	2675550.00	3234379.00	3253220.00	2517785.00	3779915.00	3178350.00	3184461.00	1843641.00	1884920.00	1952803.00	2079559.00	2916975.00	249530.80	495023.50	339626.20	1555892.00	1567711.00	1432340.00	202160.70	139415.40	328352.80	1725126.00	1329690.00	640335.70
Xanthine	836157.40	889925.80	638742.90	541916.30	684555.80	741037.00	1024153.00	1005127.00	1075833.00	1040501.00	901921.70	1304958.00	820488.80	1134198.00	1324635.00	226205.40	313094.80	372162.50	1115972.00	1083533.00	784869.50	171099.80	187608.70	395248.10	493509.40	490792.90	548876.80
(S)(+)-Allantoin	64540.51	35621.88	34636.79	93004.06	83360.71	64802.34	115192.20	101380.40	105313.90	68204.79	99681.04	106323.10	54626.05	48679.81	47954.93	23989.99	30181.66	27078.05	44219.66	50724.25	58107.04	28306.75	28240.35	69656.73	60961.41	94785.54	58327.99
Urate	217772.20	99533.62	133352.00	53420.32	45127.01	92470.10	164223.10	179349.40	193362.10	249348.00	80541.55	261928.30	156031.30	92304.41	232175.90	29137.30	45010.82	116134.60	155711.70	303520.80	115949.40	92920.99	76490.79	142257.70	86866.61	68732.73	139662.20
3',5'-Cyclic IMP	11179900.00	11273540.00	12299580.00	13517810.00	14127680.00	21266080.00	15014320.00	19392010.00	22280140.00	14354980.00	18092040.00	18939380.00	17906050.00	17372430.00	18424830.00	17098650.00	14891190.00	22143430.00	18494640.00	19281570.00	17355520.00	18736190.00	15553940.00	28417070.00	15179080.00	18053380.00	26648820.00
5-6-Dihydrothymine	106411.10	94973.66	82705.47	89264.75	71830.12	89638.07	86304.34	132935.40	90784.90	108378.20	90502.56	77052.28	89594.62	83784.37	84629.47	105889.30	123727.70	144042.60	100060.10	77851.25	109301.70	97180.19	109586.00	127780.40	34401.41	66801.23	52074.78
Nicotinate ribonucleotide	148336.20	153571.70	176095.70	141420.70	183298.10	214414.40	136039.10	152700.70	159376.60	130013.30	116870.00	145605.80	89328.43	79631.26	98232.77	153084.20	142042.10	155252.40	57236.78	101043.40	147269.80	178113.60	186094.40	206732.10	101339.40	98213.34	117895.70
UDP-glucose	152899.30	179795.60	182594.60	148097.60	181608.50	170701.30	150010.10	170362.70	181726.80	136832.80	132684.30	127667.50	282108.70	209015.40	231753.80	212978.90	165772.40	234873.10	343778.80	395534.80	411445.00	192339.90	183180.00	277805.60	143287.30	208716.00	184499.10
ADP-D-ribose	320479.50	275063.40	326625.40	89761.66	88824.98	151156.40	208594.50	210399.90	311384.00	579241.20	478878.50	606023.00	466446.40	457845.40	497222.90	153558.50	244365.10	260801.80	361515.30	446285.70	365248.30	194511.60	257300.20	314896.40	245126.10	207753.10	300065.80
Phosphate	38357880.00	41358370.00	41588570.00	41643040.00	43536700.00	52461230.00	58286430.00	54454800.00	72103100.00	52841410.00	53581540.00	62605660.00	68092840.00	57418140.00	51031990.00	37736930.00	53718620.00	38714290.00	57810860.00	66684790.00	64379550.00	46076740.00	35698280.00	67221830.00	58900560.00	52676270.00	87243460.00
Diphosphate	2941177.00	3036252.00	2378468.00	2626418.00	3301289.00	3558435.00	4406508.00	4596819.00	5650228.00	4455220.00	3909504.00	4307714.00	5381082.00	5035772.00	5153148.00	2418496.00	5314202.00	4045397.00	5301978.00	4703076.00	4697136.00	3932025.00	2385346.00	5130569.00	3949874.00	5476838.00	7589886.00
D-Glucose	344558.60	207458.50	259724.90	414732.00	422819.00	564566.10	557176.10	798111.50	1077890.00	453709.80	323155.30	357912.00	305252.50	221218.20	280358.10	640446.10	635202.10	622389.50	564536.90	428665.80	814252.10	512008.20	980444.20	1983796.00	342640.00	458755.30	428005.10
D-Fructose 1-6-bisphosphate	0.00	0.00	4399.16	25276.80	37391.28	60126.04	48920.38	38337.60	46266.83	13758.67	24974.47	11938.24	11312.95	0.00	11714.73	0.00	0.00	0.00	17716.14	11668.95	53475.53	0.00	0.00	8890.99	9845.06	50503.09	11328.57
D-Glyceraldehyde 3-phosphate/Glycerone phosphate	138874.50	138586.30	113986.00	638123.80	708111.80	532261.60	574205.40	481272.70	717233.90	526979.10	515356.50	704070.20	90141.25	210279.90	171433.00	30050.26	45041.77	43936.50	225380.30	190441.60	205573.90	47122.31	29385.40	41062.40	214990.60	339338.30	478806.40
2/3-Phospho-D-glycerate	248968.30	312091.90	296997.50	173593.50	243199.00	175293.40	213675.80	207394.50	240800.40	244985.10	261462.60	323543.10	755242.80	526385.70	721792.30	70180.21	104300.50	101742.50	685105.70	571896.80	1117548.00	104457.80	98118.55	337661.80	329610.70	389988.00	417240.10
Pyruvate	383495.20	371727.80	283684.90	617630.90	362970.60	428763.00	347166.50	294698.30	265005.70	138309.20	349952.50	385569.60	228501.20	291304.50	244223.10	203056.50	267044.70	234404.20	340966.10	342667.60	294285.10	282443.30	192661.40	417848.10	353038.70	297569.80	337809.10
Lactate	2714630.00	2475517.00	1896997.00	3581926.00	3183320.00	2545326.00	5109394.00	3216657.00	3280923.00	6412154.00	5894600.00	6800886.00	6514922.00	4562558.00	3516138.00	3424091.00	4194834.00	4359230.00	3943085.00	5492514.00	4303472.00	2254339.00	2622716.00	6905184.00	13975740.00	9071356.00	10672740.00
Maltose	65624.62	33193.94	44190.18	32145.09	48146.89	31281.90	28877.99	17373.51	27533.31	30956.56	32989.04	38562.19	25161.79	31701.90	22827.08	41432.77	42898.10	86163.04	27378.49	429271.10	30762.55	37669.34	39894.70	38424.37	51922.85	31139.69	26928.85
Mannitol/Sorbitol	144012.30	117209.40	119549.50	173474.80	190144.60	211896.70	224862.60	277219.70	408063.70	277816.10	153226.10	267511.80	84034.40	119697.80	143064.00	125609.60	181563.10	181984.10	120937.20	128532.40	154793.90	106168.20	136355.50	180045.00	191032.30	179129.80	146609.10
D-Ribose	65574.40	69223.38	77180.54	38419.80	52839.18	69793.24	70716.18	83325.16	67408.30	83479.04	66073.09	72683.07	38975.97	23516.15	48706.53	91184.03	138406.50	112553.60	65967.84	63533.07	97894.68	91384.97	73102.62	122119.80	11381.11	35370.91	22653.50
D-Arabitol	12513.36	14686.41	23162.87	29581.37	42830.94	49544.89	45914.29	70644.02	63193.97	56817.61	39925.52	66783.72	16787.42	18870.10	37704.86	13880.79	16745.00	13612.57	15770.02	32383.18	31819.60	3931.97	9136.43	34509.96	29668.52	46961.74	17598.48
Citrate	328670.70	547177.40	382659.50	924228.50	971423.20	1111336.00	777159.10	938999.80	1315360.00	916094.20	731727.90	878044.20	574594.40	607649.10	618551.60	174231.50	267087.30	263337.80	760636.20	739052.70	635231.70	300380.80	256555.00	472429.60	691435.80	823506.80	1299523.00
2-Oxoglutarate	179605.60	206171.80	154239.80	71103.84	65892.02	61778.03	74186.90	72578.62	155062.90	131585.70	141580.10	147223.60	59824.73	73257.36	44207.59	3423.09	10949.96	15913.51	25042.57	31649.61	24776.20	0.00	5866.93	17612.20	71153.99	94212.70	128740.80
Fumarate	146988.90	231675.20	118760.60	230780.10	283758.80	240095.50	256969.10	441307.10	419028.10	185191.00	212037.60	170772.10	209476.00	223867.40	215467.20	49229.59	45914.50	47879.83	934748.30	894765.20	1022079.00	71456.10	67138.60	141441.80	192095.20	191395.60	217828.70
Malate	2741964.00	3785823.00	2275807.00	3864188.00	4322997.00	3634598.00	4541532.00	8013126.00	7811414.00	3751058.00	3439205.00	2819539.00	2899739.00	4601400.00	3264947.00	519290.70	549748.80	719084.00	18073840.00	17136740.00	11108520.00	1358194.00	1125491.00	2365716.00	2514266.00	3028221.00	3672436.00
Oxaloacetate	32861.01	18613.98	24182.77	9421.16	19662.27	17762.10	25987.04	12646.60	7066.88	18162.01	12766.74	13275.51	20481.15	13199.58	14372.41	14120.74	19311.00	21421.04	25555.36	26995.02	22127.89	11900.52	16763.35	27406.88	22906.09	25765.90	41160.26
2-Hydroxyglutarate/Citramalate	707940.00	964989.20	661932.20	471897.70	562091.90	499433.70	514541.00	485413.60	865413.80	954769.50	891859.20	967102.80	700631.40	1298994.00	789085.00	56319.04	105084.10	112098.60	453316.20	402224.00	311549.70	73578.69	65382.80	54738.27	888822.00	902466.40	1119930.00
6-Phospho-D-gluconate	3791.88	4408.04	9632.52	0.00	0.00	3197.63	0.00	0.00	0.00	0.00	4787.67	15142.13	8043.25	5934.95	8468.21	0.00	8434.44	0.00	5738.78	11944.64	14772.21	0.00	5151.78	9377.25	2525.44	6254.43	8134.48
D-Glucono-1-5-lactone 6-phosphate	8056.34	10244.80	7890.84	8874.03	8652.63	32964.56	19478.32	9629.71	16239.50	8669.11	20043.94	29272.34	9130.76	11999.20	12570.05	0.00	0.00	6674.64	5851.52	8678.00	10416.70	9729.17	12676.73	20836.38	10210.65	14324.10	14418.15
Sedoheptulose 1/7-phosphate	56533.83	63694.41	47216.23	107926.10	97023.95	102097.50	81793.91	83864.93	121063.10	69170.24	79652.12	91919.50	64607.14	69170.21	63232.64	1955.38	7433.61	17832.46	54706.51	73497.12	51824.34	4986.90	5934.30	33529.09	115957.10	126002.50	111647.10
alpha-D-Ribose 1-phosphate	1695577.00	1640898.00	1257417.00	1772970.00	2366082.00	1948938.00	1748571.00	2432096.00	2623013.00	2265558.00	1587634.00	1755854.00	1520090.00	1716540.00	1437910.00	424295.30	697354.80	681564.20	1466346.00	1599130.00	1239819.00	624374.50	562759.80	861848.70	1656172.00	1500852.00	1826805.00
Glutathione	6566548.00	4340426.00	6006446.00	6994724.00	4983350.00	6035870.00	6701640.00	9566405.00	6797606.00	5156343.00	4036202.00	5997762.00	6222394.00	7962420.00	8107786.00	1540627.00	2120428.00	2863829.00	6188178.00	6739022.00	5806206.00	1705637.00	1529983.00	2446758.00	4159723.00	3342627.00	4135719.00
Ascorbate	958636.30	849819.90	715800.80	348781.10	341038.20	454106.40	339706.30	514643.40	601612.10	679137.50	821481.40	869204.80	453484.20	451675.20	379615.70	32704.02	23374.30	38417.33	537663.20	748017.10	693957.90	45520.31	33210.89	99578.15	312061.80	566275.10	425154.80
Dehydroascorbate	27319.47	53350.38	30627.74	65015.14	55607.86	46214.56	41353.82	75598.55	82902.11	39051.69	73618.46	44315.82	53077.46	52015.83	55496.80	4431.44	11658.60	9670.45	55901.20	40971.49	37603.58	4256.83	5222.25	13178.63	20782.75	32667.96	32394.42
L-gamma-Glutamyl-L-hypoglycin	0.00	0.00	0.00	0.00	0.00	0.00	0.00	2819.01	0.00	0.00	0.00	0.00	0.00	0.00	0.00	0.00	9178.18	4824.78	0.00	0.00	0.00	12931.28	5180.63	9972.61	0.00	0.00	0.00
3-Phosphonooxypyruvate	120986.00	58160.08	76919.65	82301.84	52189.15	102522.90	59678.95	93986.06	113976.20	128274.30	46566.91	166431.10	73651.04	88069.12	94123.94	39983.12	41538.20	47455.81	77507.76	117738.20	80237.50	54968.55	62033.92	72855.00	82981.69	76757.23	69410.12
Dihydrofolate	0.00	0.00	0.00	3286.30	4303.98	1909.93	4818.29	3813.76	3289.19	0.00	7285.80	2447.00	0.00	4599.53	0.00	1705.48	0.00	0.00	4372.43	2835.17	1394.01	1404.71	2127.08	0.00	5143.58	10340.61	4981.48
Argininosuccinate	3837.90	14622.49	3068.56	5645.99	26129.44	10558.40	9461.85	20872.79	20794.08	6619.26	13467.81	5546.19	8683.57	3639.70	0.00	14587.08	15009.88	9335.82	88458.20	118023.40	87309.33	16313.59	4826.37	11561.59	3955.78	7744.20	17205.06
N-Acetylneuraminate	4507280.00	4687606.00	4362980.00	5543117.00	4530562.00	4735792.00	7230892.00	8212974.00	8504183.00	6112372.00	5889446.00	8025098.00	3497631.00	3722061.00	3614045.00	685604.90	1004656.00	1271943.00	4351674.00	5408406.00	5105242.00	1632314.00	1058793.00	1814180.00	3312694.00	2573679.00	2713894.00
alpha-D-Glucosamine 1-phosphate	50209.42	61617.14	81096.09	48433.54	56593.86	64676.49	52821.45	49790.86	86999.70	50562.97	45860.70	60555.02	47599.20	82357.15	42737.16	20547.59	23892.74	43152.02	68157.62	57388.14	45528.17	21087.59	10508.60	10116.96	40625.22	43445.34	47419.47
1-4-beta-D-Xylan	703072.70	755589.80	448469.30	424052.40	508930.50	466275.30	569068.90	406025.50	817797.00	763893.30	604442.90	672548.80	982394.80	1389790.00	1231016.00	116953.30	143370.80	205038.50	449709.70	354373.00	286967.90	43405.52	42362.78	66338.12	709418.50	883271.80	1063836.00
UDP-N-acetyl-D-glucosamine	167421.20	207692.30	263973.20	300955.90	279357.00	380399.80	240896.20	291491.90	348716.10	165775.30	185637.60	206421.50	271286.30	229752.90	249700.70	192937.60	170288.80	215038.50	176718.60	246775.50	214082.00	165782.10	155821.80	200760.00	160721.50	185546.50	188658.50
CMP-N-acetylneuraminate	104313.90	123146.00	154339.80	149793.20	146610.90	191244.90	221445.40	272520.80	211117.50	235885.00	290315.70	279970.70	166980.20	165112.90	175185.00	57718.70	46124.91	56335.44	151290.20	173122.40	157946.70	71292.50	52204.00	71837.35	99602.95	129580.10	133202.40
Phosphocreatine	38014.69	42936.59	31822.92	131067.90	62663.66	72806.84	53551.18	69407.02	77597.70	64520.73	67245.35	97869.15	88923.56	22159.61	62719.16	68283.55	49296.79	84404.37	140774.30	111689.00	107448.00	43479.75	34046.27	51063.39	132612.60	210943.10	176199.80
5-6-Dihydrouracil	178891.40	171849.80	200480.60	190625.40	212515.10	174436.10	236512.20	338850.80	229516.20	277624.50	0.00	237558.40	236035.50	169663.20	210072.10	211040.40	214960.80	220753.10	214339.10	197904.90	192470.40	213688.80	175989.10	250799.40	162660.50	159007.90	184233.80
Taurine	15412780.00	16562980.00	9083695.00	12545320.00	9402632.00	14001360.00	9165241.00	20220690.00	11605550.00	16166570.00	13168460.00	12353400.00	26355430.00	18695580.00	34118240.00	4957730.00	5227613.00	8044510.00	22132770.00	18532760.00	19598070.00	4513164.00	4234428.00	7759508.00	13256420.00	15351180.00	16480350.00
Glycerol 3-phosphate	124551.70	100552.10	99184.81	186551.90	242615.90	221259.60	149362.20	127117.20	167932.20	148034.50	119404.10	122650.50	144571.10	218818.10	192548.50	90965.09	45148.71	76424.52	158485.90	240497.30	120730.20	55917.82	82101.38	90076.15	184056.50	88625.77	155718.30
Ethanolamine phosphate	4004515.00	3168347.00	3288149.00	6557168.00	4175919.00	4871194.00	4769210.00	8320384.00	6444902.00	4616714.00	5199264.00	6395318.00	3820907.00	4564866.00	4120853.00	525601.10	1032150.00	940076.80	3846005.00	4360632.00	3527784.00	607475.90	571565.80	1195984.00	3083354.00	2166064.00	2476943.00
N-Methylethanolamine phosphate	34759.90	20573.22	29231.66	96261.46	37833.94	76474.08	98710.77	153424.00	138319.90	155958.10	144209.70	145896.50	66378.88	72677.14	67420.72	5965.55	15429.63	14210.64	141438.20	143114.40	151546.30	21635.50	25424.02	21819.58	88206.99	70165.41	59172.25
Heptanoic acid	126989.20	236822.80	224105.40	323755.40	443691.70	243772.00	298085.20	336314.80	279971.50	348327.90	339335.30	135528.60	325455.50	247066.80	351323.10	273210.00	271670.30	360410.50	431937.90	364289.20	335184.20	329247.70	194895.40	250169.50	275056.00	401749.50	419328.70
Octanoic acid (caprylic acid)	182541.00	345834.60	215217.00	647546.20	326408.90	354761.20	292805.50	288656.30	474120.30	283476.50	210056.90	169918.70	293874.40	310453.50	504268.00	382816.50	257777.30	653455.80	279509.00	347892.00	277738.80	214493.20	202398.00	259378.80	356875.50	304547.90	237052.70
Nonanoic acid (pelargonic acid)	388941.30	707884.40	1092200.00	1167960.00	613283.70	793748.70	864151.50	734076.40	965200.70	629205.60	766539.80	330531.30	791178.00	621630.80	958854.30	691092.80	1380226.00	736104.30	991747.80	468531.80	619058.50	459765.20	798763.70	650046.90	715048.70	1023883.00	642980.30
Decanoic acid (capric acid)	501592.30	598253.90	371115.20	591075.80	483169.90	441189.00	363419.20	656616.90	451524.60	282369.60	672568.30	525329.10	878572.10	467708.30	1030398.00	497604.80	782095.40	615727.10	479927.30	352303.30	735320.50	378024.00	546297.90	385975.70	465204.70	485030.80	402478.30
Tetradecanoic acid (myristic acid)	401352.90	382363.20	684546.30	542331.90	568575.70	597046.10	1540357.00	622726.80	703496.00	498139.70	295279.30	416178.40	573060.10	558938.20	473875.20	560058.30	640064.90	373425.50	479392.50	492443.30	616519.60	406523.70	484249.80	274278.60	525146.70	495216.10	497597.20
Hexadecanoic acid (palmitic acid)	3230303.00	3661972.00	3898777.00	8456644.00	4977522.00	3789256.00	2677244.00	6983108.00	4384942.00	4904914.00	2005531.00	2819923.00	4225750.00	3568905.00	7141278.00	4500654.00	3360505.00	4164798.00	2569284.00	7276652.00	2200824.00	5672400.00	4266237.00	6462196.00	4824458.00	4683766.00	5653952.00
Octadecanoic acid (stearic acid)	1413977.00	2774269.00	708834.00	1650076.00	1707585.00	839889.60	1066835.00	1966890.00	1122467.00	1842427.00	1198555.00	1263296.00	2397599.00	1546375.00	1245119.00	2063864.00	1902848.00	1098750.00	1173201.00	1122120.00	1858093.00	1387029.00	1205399.00	937843.80	854457.50	931461.50	1968948.00
Tetradecenoic acid (myristoleic acid)	36040.11	33723.78	62470.50	29299.45	69300.15	32308.90	27688.04	41935.27	20651.08	27604.48	25074.89	35624.10	38362.35	47280.09	32536.21	32841.17	43178.12	29769.19	27979.80	31144.62	40325.93	27019.42	35864.29	38552.80	30709.07	29493.52	29863.90
Hexadecenoic acid (Palmitoleic acid)	186098.90	180015.10	239704.20	289453.00	501529.30	368441.70	260122.70	287371.20	373397.30	234266.40	259094.60	258020.60	282094.30	291006.60	269651.00	146239.00	262627.70	243174.90	326366.50	279187.50	341599.40	262040.70	122341.80	162674.10	304568.60	222869.60	342120.50
Octadecenoic acid (Oleic acid)	504655.90	662145.50	748927.20	717391.50	1068181.00	1013265.00	1828614.00	1282320.00	1291287.00	759086.00	915481.10	816356.60	1285562.00	609839.20	1657144.00	421590.30	469959.20	358160.00	697220.40	1207309.00	1179927.00	609862.60	917004.00	852384.80	725767.80	496346.50	1756523.00
Linoleic acid ((9Z,12Z)-Octadecadienoic acid)	74393.75	99277.88	92941.18	281105.80	114122.90	166114.50	143173.70	156312.50	333856.30	154735.90	109809.50	316569.10	156502.80	100170.80	94848.85	82770.79	92890.90	175560.20	117780.10	168874.00	62600.57	138882.30	85578.34	146676.00	170978.20	139427.60	111321.20
a-Linolenic acid (Octadecatrienoic acid)	2677.19	7990.14	5801.37	4178.24	6375.79	2441.31	5499.95	8489.70	8439.60	4118.03	2842.81	4990.61	2006.17	3794.61	1500.09	0.00	1836.79	4380.08	4372.98	2694.46	1287.03	0.00	0.00	4399.16	5722.83	8551.54	4338.61
Arachidonic acid (Eicosatetraenoic acid)	540528.60	500800.40	945941.40	548033.60	383556.50	730645.20	2040786.00	966803.20	926490.80	840628.50	377234.30	625296.80	477139.20	683043.90	515676.50	334913.30	595092.80	257434.80	292798.30	381677.20	381021.60	192760.40	211881.50	129541.60	321005.00	279477.10	394511.70
Docosahexaenoic acid	252256.40	295849.70	411208.70	155686.20	265690.00	238150.40	355522.30	440896.70	503128.00	213489.60	181949.30	423830.00	179679.80	194673.20	252272.20	197571.80	226855.40	190280.90	310375.60	173500.80	164926.00	174650.40	132237.70	138179.90	263502.70	450622.50	245810.90
Eicosapentaenoic acid	259458.30	133207.30	282921.70	243391.20	163741.20	247343.40	125626.40	136731.50	405688.10	142287.60	87118.07	219190.70	174318.80	177461.30	393540.80	120450.80	62101.19	76900.96	76782.72	59209.68	56320.27	63290.05	63802.66	28545.45	41445.62	89732.52	108986.30
Itaconate	4239934.00	5313184.00	3483441.00	8156468.00	8088204.00	9339301.00	11772260.00	11761020.00	15659860.00	12792320.00	11925760.00	12844210.00	9761294.00	12875870.00	12077070.00	1207800.00	1821579.00	2045626.00	5351718.00	4108022.00	4488063.00	1608181.00	1167380.00	2620739.00	11705750.00	14472080.00	17974230.00
Citrate 13C2	0	0	0	0	0	0	0	0	0	0	0	0	6900.470794	0	0	0	0	0	18530.43871	24097.42644	29017.53071	0	0	0	24875.54566	17315.31438	24774.11781
2-Oxoglutarate 13C3	0	0	0	0	0	0	0	0	0	0	0	0	54093.46	363445.2	103924.9	232753.4	101116.1	187766.1	201817.8	244080.2	56250.77	258519.2	280149	254160.4	353458.4	203166.7	258689.2
2-Oxoglutarate 13C5	0	0	0	0	0	0	0	0	0	0	0	0	25632.47	23093.11	7474.958	6484.134	13266.47	10889.76	24596.1	36350.98	12024	36275.97	13666.3	12159.87	12087.12	16815.61	27202.45
Itaconate 13C1	0	0	0	0	0	0	0	0	0	0	0	0	12786.73	0	0	0	0	25287.87	189348.91	169023.59	203313.535	47903.645	17117.69	8268.655	223440.65	303139.6	340133.35
Itaconate 13C2	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	108668.8531	82572.26345	72126.15943	1495.625475	13929.0455	7054.614525	69412.80625	95527.958	140383.4543
Itaconate 13C3	0	0	0	0	0	0	0	0	0	0	0	0	867612.7	1377729	950155.6	1363064	1208742	1541673	1713709	1935040	1650165	765649.3	705280.8	1393967	1145404	1041144	926176.2
Itaconate 13C4	0	0	0	0	0	0	0	0	0	0	0	0	24516.04	30485.01	35819.52	39767.62	54543.23	65539.98	286121.5	238350.5	190509.8	27656.38	35523.6	60845.24	198209.5	229753.2	309908.6
Succinate 13C4	0	0	0	0	0	0	0	0	0	0	0	0	401274	382598.7	396831.8	272134.5	413191.8	332756.4	276625.1	244140.5	383983	251986.4	227206.7	489268.4	378256	507760.3	352497.2
Malate 13C1	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	4819.6228	15689.224	112767.44	94211.94	7060.32	8688.204	0	18981.796	0	16634.676	7743.516
Malate 13C2	0	0	0	0	0	0	0	0	0	0	0	0	0	0	2260.417608	4107.260205	5256.969323	5901.319376	239121.8458	223777.0714	151471.3053	8993.806416	2787.132424	25822.02382	35777.99102	33609.97414	69029.0639
Malate 13C3	0	0	0	0	0	0	0	0	0	0	0	0	604.4818	1046.911	1101.311	962.4062	996.3853	2689.377	182874.5	166637.2	111127.7	2971.204	1127.48	2829.764	5058.423	701.2951	2555.856
Malate 13C4	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	1964.208	0	0	899969.3	862266.9	538192.3	9554.743	8083.208	27275.65	43253.81	42233.77	62528.3
Pyruvate 13C1	0	0	0	0	0	0	0	0	0	0	0	0	4249.2204	0	6593.7277	4593.2855	1351.9649	468.1184	8331.0987	10873.4792	5869.7217	4368.9111	8406.2238	10304.8627	2852.5829	1768.4466	352.5697
Lactate 13C1	0	0	0	0	0	0	0	0	0	0	0	0	7157.874	0	0	21998.997	7403.778	13118.91	16852.995	0	59.124	11717.033	12418.212	0	27889.88	35856.452	29057.78
ADP 13C1	0	0	0	0	0	0	0	0	0	0	0	0	674120.6249	738078.5999	898491.4396	674276.6293	1044618.275	785671.3209	654981.0074	505020.649	857230.5068	582054.5513	407492.1064	922748.8199	522543.9138	1137719.449	908901.9246
ADP 13C2	0	0	0	0	0	0	0	0	0	0	0	0	63226.54274	76729.61099	98666.05336	58224.73922	105019.6703	81819.9993	65434.56481	51120.80439	101847.9737	58466.91464	54146.4677	93000.02819	60540.89452	115167.8594	109458.1057
AMP 13C2	0	0	0	0	0	0	0	0	0	0	0	0	4711.8476	11969.7439	29989.689	0	0	716.2909	20723.7904	24756.9406	11443.342	9094.1042	842.16596	8909.1411	20939.7222	20544.98	15681.081
AMP 13C4	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	37367.69	32003.19	16714.16	2558.278	0	0	36033.75	22748.3	32549.13
AMP 13C5	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	227644.2	228072.1	172965.9	18967.53	18666.96	22659.29	264218.8	223305.6	257278.5
AMP 13C6	0	0	0	0	0	0	0	0	0	0	0	0	4285.8	16228.11	3919.629	7632.064	4091.044	2457.001	18714.66	16869.25	12957.44	0	0	0	17550.43	14239.08	13706.58
AMP 13C7	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	5784.916	3144.555	2879.189	18924.67	19246.14	16567.35	6671.854	5465.322	4405.009	5589.908	4162.786	4503.246
AMP 13C8	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	25776.55	21385.66	20703.41	0	0	6549.546	16679.63	11526.69	10165.21
AMP 13C9	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	85774.48	94917.85	69445.91	0	0	2886.912	38566.34	30311.69	37879.59
AMP 13C10	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	520266.7	518851.1	424206	24591.87	11379.12	24240.76	191716.6	173352.7	166875.6
Hexose phosphate 13C6	0	0	0	0	0	0	0	0	0	0	0	0	0	0	922.9222	0	4550.51	0	2200.61	2418.513	0	0	1816.691	0	0	0	0
MS_METABOLITE_DATA_END
#METABOLITES
METABOLITES_START
metabolite_name	KEGG ID	m/z	RT
ADP	C00008	426.0217	0.605
AMP	C00020	346.0554	0.648
GMP	C00144	362.0506	0.617
UMP	C00105	323.0281	0.609
IDP	C00104	427.0067	0.577
IMP	C00130	347.0394	0.618
Inosine	C00294	267.0731	0.709
Xanthine	C00385	151.0248	0.689
(S)(+)-Allantoin	C02350	157.0354	0.681
Urate	C00366	167.0198	0.641
3',5'-Cyclic IMP	C00943	329.0298	0.545
5-6-Dihydrothymine	C00906	127.0498	0.654
Nicotinate ribonucleotide	C01185	335.0468	0.551
UDP-glucose	C00029	565.0469	0.552
ADP-D-ribose	C01882	558.0630	0.590
Phosphate	C00009	96.9679	0.604
Diphosphate	C00013	176.9346	0.600
D-Glucose	C00031	179.0550	0.662
D-Fructose 1-6-bisphosphate	C00354	338.9883	0.558
D-Glyceraldehyde 3-phosphate/Glycerone phosphate	C00118	168.9892	0.591
2/3-Phospho-D-glycerate	C00631	184.9845	0.572
Pyruvate	C00022	87.0072	0.615
Lactate	C01432	89.0228	0.618
Maltose	C00208	341.1096	0.670
Mannitol/Sorbitol	C00392/C00794	181.0702	0.674
D-Ribose	C00121	149.0451	0.682
D-Arabitol	C01904	151.0599	0.675
Citrate	C00158	191.0186	0.594
2-Oxoglutarate	C00026	145.0129	0.593
Fumarate	C00122	115.0032	0.588
Malate	C00149	133.0127	0.589
Oxaloacetate	C00036	131.0001	0.609
2-Hydroxyglutarate/Citramalate	C02630	147.0287	0.600
6-Phospho-D-gluconate	C00345	275.0173	0.569
D-Glucono-1-5-lactone 6-phosphate	C01236	257.0070	0.579
Sedoheptulose 1/7-phosphate	C06222	289.0328	0.593
alpha-D-Ribose 1-phosphate	C00620	229.0111	0.591
Glutathione	C00051	306.0762	0.621
Ascorbate	C00072	175.0236	0.566
Dehydroascorbate	C05422	173.0079	0.581
L-gamma-Glutamyl-L-hypoglycin	C08280	269.1116	0.695
3-Phosphonooxypyruvate	C03232	182.9668	0.780
Dihydrofolate	C00415	442.1559	0.681
Argininosuccinate	C03406	289.1151	0.600
N-Acetylneuraminate	C00270	308.0983	0.609
alpha-D-Glucosamine 1-phosphate	C06156	258.0380	0.605
1-4-beta-D-Xylan	C02352	131.0334	0.606
UDP-N-acetyl-D-glucosamine	C00043	606.0740	0.553
CMP-N-acetylneuraminate	C00128	613.1394	0.551
Phosphocreatine	C02305	210.0276	0.561
5-6-Dihydrouracil	C00429	113.0341	0.597
Taurine	C00245	124.0059	0.652
Glycerol 3-phosphate	C00093	171.0051	0.607
Ethanolamine phosphate	C00346	140.0104	0.617
N-Methylethanolamine phosphate	C01210	154.0261	0.623
Heptanoic acid	C17714	129.0907	1.891
Octanoic acid (caprylic acid)	C06423	143.1064	2.071
Nonanoic acid (pelargonic acid)	C01601	157.1221	2.158
Decanoic acid (capric acid)	C01571	171.1378	2.240
Tetradecanoic acid (myristic acid)	C06424	227.2011	2.680
Hexadecanoic acid (palmitic acid)	C00249	255.2325	3.056
Octadecanoic acid (stearic acid)	C01530	283.2638	3.619
Tetradecenoic acid (myristoleic acid)	C08322	225.1855	2.476
Hexadecenoic acid (Palmitoleic acid)	C08362	253.2168	2.732
Octadecenoic acid (Oleic acid)	C00712	281.2482	3.092
Linoleic acid ((9Z,12Z)-Octadecadienoic acid)	C01595	279.2325	2.775
a-Linolenic acid (Octadecatrienoic acid)	C06427	277.2169	2.590
Arachidonic acid (Eicosatetraenoic acid)	C00219	303.2325	2.679
Docosahexaenoic acid	C06429	327.2325	2.587
Eicosapentaenoic acid	C06428	301.2169	2.509
Itaconate	C00490	129.0178	0.594
Citrate 13C2	C00158	193.0243	0.5869578
2-Oxoglutarate 13C3	C00026	148.0265	0.6808727
2-Oxoglutarate 13C5	C00026	150.0298	0.6131334
Itaconate 13C1	C00490	130.0217	0.5866438
Itaconate 13C2	C00490	131.0245	0.5897642
Itaconate 13C3	C00490	132.0287	0.5977243
Itaconate 13C4	C00490	133.0319	0.5961062
Succinate 13C4	C00042	121.0299	0.6802999
Malate 13C1	C00149	134.0162	0.5862014
Malate 13C2	C00149	135.0188	0.5929192
Malate 13C3	C00149	136.0237	0.5553871
Malate 13C4	C00149	137.0261	0.5994042
Pyruvate 13C1	C00022	88.01049	0.6419379
Lactate 13C1	C01432	90.02612	0.6192572
ADP 13C1	C00008	427.0182	0.7369176
ADP 13C2	C00008	428.0216	0.7432361
AMP 13C2	C00020	348.0616	0.6652799
AMP 13C4	C00020	350.0692	0.6453673
AMP 13C5	C00020	351.0723	0.648688
AMP 13C6	C00020	352.0795	0.6286229
AMP 13C7	C00020	353.0824	0.6618488
AMP 13C8	C00020	354.0818	0.6466244
AMP 13C9	C00020	355.0873	0.6626313
AMP 13C10	C00020	356.0903	0.6544209
Hexose phosphate 13C6	C02965	265.0414	0.6382095
METABOLITES_END
#END